Nathan Joseph, Chyna Ellis, Danielle Sellers and Craig Lawson were all axed in this evening's episode in a dramatic shake up.
They were among the six least popular Islanders alongside Jonny and Tyla.
As the two contestants with the fewest votes, Nathan and Chyna were immediately axed. The most popular two - Marcel and Montana - then had to pick which of the next two least popular islanders should leave.
Montana sent Craig home over Jonny while Marcel sent Danielle home over Tyla.
Speaking after their exits, Danielle and Nathan have both taken aim at 'fake' Kem and Amber.
"I went for Kem at first and he said he would couple up with me out of anyone," Danielle said. "I didn’t show him any attention for three to four hours and he was already onto the next girl."
She told the Daily Mirror: "I don’t think he wanted to see Amber with anyone else."
Meanwhile, Nathan claimed: "If Amber didn’t choose me and went home Kem would be cracking on with Chyna. Rather than a case of wanting Amber he doesn’t want to see her with anyone else.
"They’re both young and when you’re younger it’s easy to say I’m in love. There is emotion there but I can’t see it."
He suggested: "I think it will get a bit boring and tedious - they’ll make up, have a row, then say they love each other.
"Chris Hughes and Olivia Attwood said they're so sick of the situation now. "
Love Island 2017 continues nightly on ITV2.